What question did this study set out to answer?

This research aims to connect small-scale lithiation mechanisms with the larger performance of silicon anodes in lithium-ion cells.

February 28, 2026EES batteries.Open Access

Bridging particle-scale lithiation mechanisms and macroscopic performance in high-energy density Si anodes via time-resolved full 3D visualisation

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This research aims to connect small-scale lithiation mechanisms with the larger performance of silicon anodes in lithium-ion cells.
Utilized 4D synchrotron nano-tomography to visualize electrode characteristics.
Assessed particle-resolved strain and deformation during lithiation processes.
Analyzed the correlation between microstructural changes and macroscopic performance.
Identified significant link between particle-scale strain and overall electrode performance.
Revealed complex chemo-mechanical interactions within high content silicon electrodes.
Provided detailed visualization of lithiation dynamics affecting battery efficiency.

Implication

Correlative 4D nano-tomography reveals insights into lithiation dynamics in silicon anodes, suggesting improved design strategies.

Abstract

Correlative 4D synchrotron nano-tomography links electrode-scale deformations with particle-resolved strain and lithiation dynamics, revealing enhanced insights into the chemo-mechanical processes of Li-ion cells with high Si content.

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Cite This Study

Häusler et al. (2026) studied this question.

synapsesocial.com/papers/69a286da0a974eb0d3c021d4 https://doi.org/10.1039/d6eb00026f

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Implication

Correlative 4D nano-tomography reveals insights into lithiation dynamics in silicon anodes, suggesting improved design strategies.

Bridging particle-scale lithiation mechanisms and macroscopic performance in high-energy density Si anodes via time-resolved full 3D visualisation

Key Points

Implication

Abstract

Discussion

Cite This Study

Bridging particle-scale lithiation mechanisms and macroscopic performance in high-energy density Si anodes via time-resolved full 3D visualisation

Key Points

Implication

Abstract

Discussion

Cite This Study

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