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March 13, 2026EES Catalysis0 citationsOpen Access

Spatially Extended Asymmetry Directs Electron Transfer and Modulates Water Oxidation Deprotonation Behavior on Dual-Atom Catalysts

JYJixuan YangYCYaxin ChengHMHao Ma

Key Points

  • The aim is to explore how local coordination asymmetry influences electron transfer and water oxidation behavior in dual-atom catalysts.
  • Introduced local coordination asymmetry via heteroatom substitution in dual-atom catalysts.
  • Analyzed changes in electronic state of metal centers based on substitution variations.
  • Evaluated effects on electron transfer and water oxidation deprotonation behavior.
  • Local coordination asymmetry significantly modulated electron transfer efficiency.
  • Water oxidation deprotonation behavior was altered due to changes in electronic states.
  • Specific substitutions led to enhanced catalytic performance.

Abstract

Introducing local coordination asymmetry through heteroatom substitution in homonuclear dual-atom catalysts (DACs) is an effective strategy to modulate the electronic state of metal centers. However, this approach often results in...

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Cite This Study

Yang et al. (2026) studied this question.

synapsesocial.com/papers/69b3abe702a1e69014ccd2cchttps://doi.org/10.1039/d5ey00362h
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