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March 14, 2026Tetrahedron LettersOpen Access

On the mechanism of ketene three-component reaction

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Authors

MCMarcelo H.R. CarvalhoMRMateus S. RozaBNBRENNO A.D. NETO

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Overview

This investigation details the mechanisms of ketene reactions, revealing key steps and implications for synthesis.

Key Points

  • The aim is to explore the mechanisms of ketene three-component reactions and their silylative variant.
  • Utilized density functional theory (DFT) calculations to analyze reaction mechanisms.
  • Conducted mass spectrometry (ESI-MS) experiments to monitor reaction pathways.
  • Identified elementary steps and divergence points in both K-3CR and SK-3CR.
  • Outlined complete reaction pathways for both K-3CR and SK-3CR.
  • Identified key intermediates and steps in the reaction mechanisms.
  • Proposed a unified framework that aligns with existing experimental data.

Cite This Study

Carvalho et al. (2026) studied this question.

synapsesocial.com/papers/69b4fa9ab39f7826a300b558https://doi.org/10.1016/j.tetlet.2026.156041
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