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This research describes a vinyl group transfer reaction in 4-vinyl-1,4-dihydropyridines, suggesting new pathways for creating fluorinated compounds.
The visible-light-driven, organophotoredox-catalyzed vinyl group transfer reaction is described. The strategic use of proaromatic, bench-stable, and readily prepared 4-vinyl-dihydropyridine (DHP) derivatives triggers the vinyl group transfer that can couple stereoselectively with fluorinated esters and amides to forge the C(sp³)-C(sp²) bond. The obtained products are transformed into diverse fluorinated scaffolds. Preliminary mechanistic investigations are outlined.
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Mandhotra et al. (2026) studied this question.
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