This research demonstrates spin crossover tuning in dinuclear complexes, indicating a role for ligand redox-state.
The spin crossover behavior in dinuclear Fe III complexes is tuned by changing the oxidation state of the bridging bis(dioxolene) ligand, with the mixed-valence form imparting an asymmetric ligand field that drives a two-step interconversion.
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Janetzki et al. (2026) studied this question.
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