Laboratory study demonstrates efficient uranium extraction in seawater environments, suggesting a durable and reusable strategy for nuclear fuel recovery.
For uranium extraction from seawater, development of new stable and reusable sorbents with high affinity and good selectivity for U(VI) is required. Herein, a new phosphate-functionalized polyethylene (denoted PO₄/PE) was synthesized via a simple Ar-jet plasma treatment of PE in concentrated H₃PO₄ and was employed in U(VI) extraction from seawater. The prepared PO₄/PE shows superior performance in the extraction of trace U(VI) from seawater. The adsorption process followed the second-order kinetics model and the Langmuir model. The maximum adsorption capacity of PO₄/PE for U(VI) reaches 173.8 mg/g at pH 8.2 and 298 K. PO₄/PE can be effectively regenerated by 0.1 mol/L Na₂CO₃ and reused well even after eight cycles. Experimental results offer a new approach for U(VI) uptake from seawater.
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