The chemical compositions of 26 metal-poor stars that exhibit strong CH and/or C2 molecular bands are determined based on high-resolution spectroscopy. We define carbon-enhanced stars taking account of the carbon abundance ratio ([C/Fe]) and the evolutionary status, which is a slight modification over previous definitions. Twenty two stars in our sample satisfy our modified definition for Carbon-Enhanced Metal-Poor (CEMP) stars. In addition, we measure Na abundances for nine other carbon-enhanced stars for which abundances of other elements have been previously reported. Combining our new sample with the results of previous work, we investigate the abundance and evolutionary status of a total of 64 CEMP stars. The following results are obtained: (1) All but one of the 37 stars with [Fe/H] ≥ −2.6 exhibit large excesses of barium ([Ba/Fe]> +0.5), while the other 27 stars with lower metallicity exhibit a large scatter in their barium abundance ratios (−1.2 < [Ba/Fe]<+3.3). (2) A correlation between the carbon and barium abundance ratios ([C/Fe] and [Ba/Fe]) is found in Ba-enhanced objects (comprising 54 stars), suggesting that the origin of the observed carbon excess in
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