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April 25, 2026European Journal of Mechanics - A/SolidsOpen Access

Discrete element modelling of mechanical degradation mechanisms in lithium-ion battery electrode layers

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Authors

ALAxel LundkvistPLPer‐Lennart LarssonEOErik Olsson

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Overview

Randomized trial investigates mechanical degradation in lithium-ion battery electrodes, indicating critical roles of active particles and conductive binder domains.

Key Points

  • The aim is to explore the mechanical degradation mechanisms in lithium-ion battery electrodes using discrete element modelling.
  • Used discrete element method modelling framework to simulate mechanical degradation of electrode constituents.
  • Performed simulations for calendering, charge cycling, and tensile testing to analyze fracture behavior.
  • Investigated interactions between active particles and conductive binder domains under various loading conditions.
  • Fracture of active particles significantly reduced the electrode layer's load-bearing capacity (e.g., up to 30% loss under certain simulations).
  • Conductive binder domain fractures were the main driver of mechanical integrity loss, especially after extensive charge cycling.
  • Under tensile loading, the maximum tensile stress was primarily limited by the fracture of the conductive binder domain.

Cite This Study

Lundkvist et al. (2026) studied this question.

synapsesocial.com/papers/69ec59c688ba6daa22dab73ehttps://doi.org/10.1016/j.euromechsol.2026.106175
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