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-Pd-Ag-N configuration, thereby modulating the electronic and geometric structures of Pd sites, which in turn benefits the adsorption and activation of substrate and lowers energy barrier for the rate-determining step of semihydrogenation, ultimately enhancing the electrocatalytic reaction. This work provides a facile and powerful strategy for the design of advanced catalysts by tuning the local coordination environment for selective catalysis.
Guo et al. (Wed,) studied this question.