High‐Security Plastic with Integrated Holographic and Phosphorescent Images

. The enhanced phosphorescence is primarily ascribed to the increase of conformational distortion and spin-orbit coupling of organic phosphors based on theoretical calculations. Eventually, the first example is demonstrated of holographic plastic with the unique capability of independently displaying holographic andphosphorescent images. This work not only provides a novel paradigm to impart added optical functions to ORTP polymer materials but also paves the way for the development of high-security optical materials to combat counterfeiting.