A negative electron affinity (NEA) was found both experimentally by photoemission spectroscopy and theoretically by ab initio calculations for the 2×{}1 reconstructed diamond (100) surface. This surface is the dominant growth surface for thin diamond films and can be obtained by chemical-vapor deposition. Various surface-preparation methods which result in a NEA are described. Theoretical results indicate that the observed NEA is associated with a monohydride-terminated surface, while the hydrogen-free surface exhibits a positive electron affinity.
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Weide et al. (1994) studied this question.
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