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May 16, 2026ACS Applied Energy Materials

Synergistic Regulation of Electrolyte Composition and Electrode Interface for Enhanced Low-Temperature Performance of Lithium-Ion Batteries

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Authors

YWYue WangBLBaodi LuLMLiang Ming

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Overview

Randomized trial demonstrates improved low-temperature performance in lithium-ion batteries, indicating potential for extreme applications.

Key Points

  • This research aims to enhance the low-temperature performance and cycling stability of lithium-ion batteries by optimizing electrolyte composition and interface characteristics.
  • Developed a systematic electrolyte containing methyl propionate, fluoroethylene carbonate, and bis(2,2,2-trifluoroethyl) ether.
  • Engineered a passivation layer (LiF and Li2CO3) on the electrode surface to reduce impedance.
  • Evaluated cycling performance using NCM523||Li and graphite||Li half-cells at varied temperatures.
  • The optimized electrolyte demonstrated a capacity retention of approximately 60% at -40 °C with a capacity of 90.5 mAh g−1 at 0.1 C.
  • The NCM523||graphite full cell showed satisfactory cycling performance at both room temperature and -20 °C.
  • High discharge capacities were achieved, measuring 104.5 and 245.2 mAh g−1 from NCM523/Li and graphite/Li half cells, respectively, under low-temperature conditions.

Cite This Study

Wang et al. (2026) studied this question.

synapsesocial.com/papers/6a080ab3a487c87a6a40ca18https://doi.org/10.1021/acsaem.6c00091
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