NiMo-MOF-Derived Carbon-Armored Ni₄Mo Alloy of an Interwoven Nanosheet Structure as an Outstanding pH-Universal Catalyst for Hydrogen Evolution Reaction at High Current Densities

for over 50 h, making it promising for applications in large-scale green hydrogen production. The success can be attributed to the unique catalyst design of a carbon-armored, composition-optimized NiMo alloy of an advantageous nanostructure of interwoven nanosheets for enhanced utilization of active sites and mass transfer of electrolytes and gaseous products, made possible with a MOF-derivation fabrication approach.