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Femtosecond pump-probe spectroscopy of the equilibrated hydrated electron has been recorded with 35 fs resolution, revealing unprecedented transient features on the 30--80 fs time scales that have been assigned to inertial solvation dynamics of the hydrated electron. These data allow for a rigorous experimental evaluation of the recently published nonadiabatic quantum molecular dynamics simulations of the adiabatic and nonadiabatic dynamics of the hydrated electron.
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Silva et al. (1998) studied this question.
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