Nonlinear optical processes, mediated by multiphoton interactions rather than single-photon response, are routinely exploited to enable a range of light-based functionalities in devices and applications. Nonlinear effects are enhanced by higher-intensity fields, which is a limiting strategy owing to potential radiation damage. An alternative strategy relies on the fluctuation redistribution typical of quantum light1–4, but experimental demonstrations at the most fundamental level have been limited. Here we report experimental nonlinear tunnelling ionization of isolated atoms, a pivotal nonlinear process that drives high-harmonic generation and forms the basis of attosecond science, boosted by quantum light—bright squeezed vacuum (BSV). A BSV light with an average pulse energy of 300 nJ achieves an effective intensity equivalent to that of a coherent light with 7.1 μJ, demonstrating a more than 20-fold quantum boost in the nonlinear effect from BSV light. This boost is revealed by matching the peaks of the photoelectron momentum spectra produced by the BSV and coherent light as measured by angular streaking. Furthermore, we demonstrate control of the effective intensity of the BSV by tuning the correlation function at fixed average pulse energy, establishing a robust method to tailor nonlinear processes by quantum statistics rather than classical intensity scaling. These findings may facilitate the development of quantum-controlled strong-field dynamics using tailored quantum light sources. Bright squeezed vacuum light boosts nonlinear atomic tunnelling ionization more than 20-fold compared with coherent light, enabling quantum control of strong-field processes without increasing classical intensity.
Jiang et al. (Wed,) studied this question.