Mapping broadband single-photon wave packets into an atomic memory

We analyze a quantum optical memory based on the off-resonant Raman interaction of a single broadband photon, copropagating with a classical control pulse, with an atomic ensemble. The conditions under which the memory can perform optimally are found, by means of a universal mode decomposition. This enables the memory efficiency to be specified in terms of a single parameter, and the control field pulse shape to be determined via a simple nonlinear scaling. We apply the same decomposition to determine the optimal configurations for read-out.