We present experimental results of two-color photoassociative ionization (TCPAI) spectroscopy in a magneto-optical trap. A probe light beam traces out the frequency (and intensity) dependence of TCPAI. By manipulating the intensities of the trap and repumper lasers we investigate the participation of different hyperfine ground-state levels and demonstrate the conditions under which molecular bound states figure in the collision intermediate.
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Bagnato et al. (1993) studied this question.
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