Control over product probabilities and channel-specific line shapes in resonant two-photon dissociation is shown to result from quantum interference effects induced by illumination with a second laser. Control over product yield and selectivity is achieved by varying the frequency of this control laser, which need not be coherent with the excitation laser. Computations on Na₂ photodissociation show that control over product selectivity is extensive.
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Chen et al. (1995) studied this question.
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