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Monolayer and multilayer Langmuir−Blodgett (LB) films of the endohedral metallofullerene Dy@C82 mixed with arachidic acid (Dy@C82/AA) were deposited onto ITO substrates from the N2/water interface. The photoelectrochemical response of the Dy@C82/AA LB films on ITO was investigated. A stable anodic photocurrent was observed, and the effects of bias voltage, light intensity, electron donor, number of layers, and O2 were studied in detail. The results indicate that electrons flow from the electrolyte through the LB film to the ITO electrode. Dy@C82/AA and C60/AA films are compared in terms of the film formation and photoelectric response. Under appropriate conditions, the Dy@C82/AA LB films exhibit a higher photocurrent quantum yield than the C60/AA films on ITO electrodes.
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Yang et al. (2001) studied this question.
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