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reduction have all been previously observed in MOFs; however, work toward a fully MOF-based approach to artificial photosynthesis remains out of reach. Discussed here are the current limitations with MOF-based approaches: diffusion through the framework, selectivity toward high value products, lack of integrated studies, and stability. These topics provide a roadmap for the future development of fully integrated MOF-based assemblies for artificial photosynthesis.
Gibbons et al. (Tue,) studied this question.