This thesis presents advancements in quantum technology through noise spectroscopy and microscopy, indicating a path toward scalability.
Quantum technology promises to be a paradigm shift in the precision, speed, and breadth of application of technology. Recent advances in the fields of quantum computing, quantum networks, and quantum sensing have been rapid, but large-scale utilization is still out of reach. This is largely due to the fragility of the individual quantum systems that this technology seeks to control and manipulate. While small demonstrators have by now shown these novel machines to work in principle, the task in the coming years will be to make them reproducible at scale. Leveraging the advanced semiconductor fabrication technology of today's classical computers, spin qubits in semiconductors such as Si/SiGe or GaAs/AlGaAs are hoped to meet this challenge. In this thesis, I present contributions in four different areas towards this overarching goal. I present an open-source software tool for Fourier-transform noise spectroscopy, improvements and characterization of a Millikelvin confocal microscope, optical measurements of electrostatic exciton traps, and a general filter-function formalism for the description of noisy quantum dynamics. I review the theory of noise spectroscopy based on Welch's method of overlapping periodograms and lay out the design of the hardware-agnostic, open-source python_spectrometer software package that facilitates interactive noise spectroscopy in everyday use. In a didactic fashion, I explore the features and capabilities of the tool and guide the reader through its operation. I then characterize a confocal microscope incorporated in a cryogen-free dilution refrigerator, applying the aforementioned noise spectroscopy tool to evaluate the displacement noise power spectral density of the system. I develop an optical technique based on a knife-edge reflectance contrast to measure the displacement noise reaching a shot-noise floor of 1 nm/√Hz. Using this technique, I determine a displacement noise RMS of 100 nm. I measure the electron temperature of a GaAs/AlGaAs quantum dot in the microscope, finding 76 mK, and demonstrate at hand of a second-order correlation measurement of a self-assembled quantum dot the setup's optical capabilities. In the experimental part of this thesis, I first provide an introduction to photoluminescence and the quantum-confined Stark effect in semiconductor quantum wells, appealing to simple analytical theory to develop an intuition for the relevant effects. I then describe the mjolnir measurement framework developed to conduct optical measurements of electrostatic exciton traps in semiconductor membranes, and present extensive measurements in search of signatures of single-photon emitters. Finally, I develop a comprehensive theoretical formalism for describing and analyzing the noisy dynamics of quantum systems based on filter functions. There, I combine the Magnus and cumulant expansions to derive a quantum-operations formulation of the dynamics under arbitrary classical noise that can be expressed in terms of filter functions capturing the susceptibility of a quantum system in response to noise at a given frequency. I present the filter_functions software package that implements the formalism and demonstrate its efficacy using several examples.
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Tobias Hangleiter (2026) studied this question.
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