This randomized trial demonstrates increased Raman enhancement using hybrid structures integrating MoS2 and gold nanospheres with optical microfibers, indicating potential for advanced sensor design.
We demonstrate a mechanism-oriented Surface-Enhanced Raman Scattering (SERS) platform based on a hybrid structure integrating monolayer molybdenum disulfide (MoS2) and gold nanospheres (AuNSs) on an optical microfiber (MF). The microfiber serves as a whispering-gallery-mode (WGM) microcavity. Monolayer MoS2, grown directly on the microfiber surface via chemical vapor deposition (CVD), provides a chemically active interface for molecular adsorption and charge-transfer-related chemical enhancement. Subsequently deposited AuNSs couple with the microfiber-supported WGM, leading to the formation of hybrid photonic–plasmonic modes. This coupling results in a narrowed scattering resonance and a localized electromagnetic hotspot near the AuNS–microfiber interface. The combined contribution of electromagnetic enhancement from the microfiber–AuNS hybrid cavity and chemical enhancement from the MoS2 layer produces discernible Raman enhancement for Rhodamine 6G (R6G) molecules under proof-of-concept measurement conditions. This work provides a useful platform for studying SERS enhancement mediated by hybrid photonic–plasmonic modes and offers guidance for the future development of optimized fiber-based SERS sensors.
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Zhao et al. (2026) studied this question.
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