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July 2, 2026Journal of the American Chemical Society

Single-Atom Migration into a Chiral Multilayer Nanocluster Architecture

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Authors

YJYuhao JinHFHao FangHPHaoyu Pan

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Overview

Randomized trial examines single-atom behavior in chiral multilayer nanoclusters, suggesting novel structural adaptability.

Key Points

  • This research investigates the migration of a single atom within chiral multilayer nanoclusters composed of copper sulfide.
  • Fabricated two enantiomeric pairs of high-nuclearity copper sulfide nanoclusters with mixed-valence configurations.
  • Utilized in situ absorption and circular dichroism spectroscopies to study transformations.
  • Conducted ex situ pair distribution function analysis to understand structural changes.
  • Single metal ion successfully migrated into the cluster core under mild reducing conditions.
  • Findings reveal the maintained atomic framework despite significant electronic structure modifications.
  • Migration process occurs as a continuous single-particle process without fragmentation.

Cite This Study

Jin et al. (2026) studied this question.

synapsesocial.com/papers/6a45fef89ed134303130fac8https://doi.org/10.1021/jacs.6c03831
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