Bulk Spin–Orbit Torque-Driven Spin Hall Nano-Oscillators Using PtBi Alloys with Engineered Crystallinity

High Resolution Image Download MS PowerPoint Slide Spin–orbit-torque-driven auto-oscillations in spin Hall nano-oscillators (SHNOs) provide a promising route toward energy-efficient, nanoscale microwave devices for neuromorphic computing and high-frequency technologies. Achieving robust oscillations requires lowering the threshold current ( I th ), governed by the spin Hall efficiency (θ SH ). Conventional approaches to enhance θ SH often involve trade-offs, such as increased resistivity and interfacial effects. Here, we demonstrate a pronounced enhancement of the bulk spin Hall effect in PtBi alloys via crystallographic engineering, achieving a 3-fold increase in θ SH from 0.07 in Pt 100.0 Bi 0.0 to 0.24 in Pt 94.0 Bi 6.0 and 0.19 in Pt 91.3 Bi 8.7, extracted from DC-bias spin-torque ferromagnetic resonance. The enhancement arises from bulk-dominated extrinsic side-jump scattering. Correspondingly, I th is reduced by 42% and 32% in 100 nm SHNOs based on Co 40 Fe 40 B 20 (3 nm)/Pt 94.0 Bi 6.0 (4 nm) and Co 40 Fe 40 B 20 (3 nm)/Pt 91.3 Bi 8.7 (4 nm), respectively. The devices exhibit narrower linewidths (∼25 MHz), enhanced quality factors (350 ≤ Q ≤ 550, ∼4× higher than Pt (Pt 100.0 Bi 0.0 )), and a 61.6% reduction in threshold power. These findings establish PtBi alloys as efficient spin Hall materials, enabling reduced power consumption for SHNO-based neuromorphic and memory technologies.