Demonstrates programmable spin polarization in coordination architectures, indicating potential for dynamic molecular systems.
)-1,1'-binaphthyl-2,2'-diylhydrogen phosphate via host-guest interactions. Magnetic circular dichroism (MCD) reveals chirality-dependent changes in electronic states, while magnetic conductive atomic force microscopy (mc-AFM) independently demonstrates spin-selective charge transport. Systematic modulation of host-guest electronic coupling enables reversible switching of spin polarization. These results demonstrate that dynamic, chirality-matched host-guest interactions emulate enzymatic stereochemical control, offering molecular-level insight and a general design principle for chiral coordination architectures with programmable spin functions.
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Wei et al. (2026) studied this question.
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