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January 1, 2022Journal of Materials Chemistry AOpen Access

Investigating dry room compatibility of sulfide solid-state electrolytes for scalable manufacturing

Yu‐Ting Chen Maxwell A. T. Marple Darren H. S. Tan So‐Yeon Ham Baharak Sayahpour Weikang Li Hedi Yang Jeong Beom Lee Hoe Jin Hah Erik A. Wu Jean‐Marie Doux Jihyun Jang Phillip Ridley Ashley Cronk Grayson Deysher Zheng Chen Ying Shirley Meng

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Key Points

The aim is to investigate the effects of moisture on sulfide solid-state electrolytes, particularly Li6PS5Cl, and the recovery process after exposure.
Analyzed the reactions of Li6PS5Cl when exposed to moisture, focusing on hydrolysis and hydration.
Assessed the recovery of the electrolyte through heat treatment after moisture exposure.
Hydrolysis and hydration of Li6PS5Cl lead to the formation of LiCl, Li2S, Li3PO4, and oxysulfides.
Partial recovery of the electrolyte is possible with heat treatment, but sulfur loss is irreversible.

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Implication

Investigations reveal the impact of moisture on sulfide solid-state electrolytes, indicating challenges for scalability.

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Cite This Study

Chen et al. (2022) studied this question.

synapsesocial.com/papers/6a62554a7581c4a485c23d92 https://doi.org/10.1039/d1ta09846b

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