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July 24, 2026Proceedings of the National Academy of Sciences

Why shear adhesion is not monotonically enhanced by stiffening

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Authors

ZDZihao DuLKLinghao KongRBRonghao Bao

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Overview

Unified framework demonstrates nonmonotonic shear adhesion behavior in elastic adhesives, suggesting optimal modulus ratios.

Key Points

  • To understand how stiffness affects shear adhesion in elastic materials through a mechanistic framework.
  • Developed an analytical solution for finite-height elastic adhesives bonded to substrates.
  • Validated the theory with systematic experiments and finite element simulations.
  • Constructed parameterized adhesion maps for optimal modulus ratios.
  • Shear adhesion shows nonmonotonic dependence on stiffness, with distinct local maxima/minima.
  • Interfacial failure is primarily driven by edge-initiated separation and opening-mode fracture.
  • Optimal modulus ratios for robust attachment and on-demand release were identified.

Cite This Study

Du et al. (2026) studied this question.

synapsesocial.com/papers/6a6301d3395161722cd1644fhttps://doi.org/10.1073/pnas.2610914123
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