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July 28, 2026Nature CommunicationsOpen Access

Highly stable quasi-solid-state initially anode-free lithium metal batteries enabled by dynamic integrated interface engineering

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Authors

YCYunyi ChenBeijing Forestry UniversityXQXitang QianHong Kong University of Science and TechnologyYLYuxiang LyuHong Kong University of Science and Technology

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Implication

Randomized trial shows enhanced cycling stability in initially anode-free lithium batteries, indicating potential for efficient energy storage.

Key Points

  • The aim is to enhance the cycling stability and energy density of initially anode-free lithium metal batteries through interface engineering.
  • Developed a dynamic integrated interface engineering strategy with an Ag-based initiator in the electrolyte.
  • Utilized in situ polymerization and Ag+-driven deposition to improve electrode-electrolyte interfacial coupling.
  • Evaluated the performance of the Cu | |LiFePO4 cell and a 2 Ah-level pouch cell.
  • The Cu | |LiFePO4 cell achieved 90% capacity retention after 200 cycles at 0.1 C.
  • The pouch cell delivered a specific energy of 467 Wh kg−1 based on total cell weight.

Cite This Study

Chen et al. (2026) studied this question.

synapsesocial.com/papers/6a6850eb2845b684d16f0047https://doi.org/10.1038/s41467-026-76060-y
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