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Mechanistic experiments demonstrate enantioselective hydrogenolysis of C–O bonds, suggesting innovative synthetic strategies.
CBD) analogs. Preliminary mechanistic experiments and DFT calculations suggested that asymmetric hydrogenolysis proceeded via an enantioselective 1,4-transfer hydrogenation initiation step, followed by an aromatization-driven remote proton transfer and skeletal rearrangement.
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Xie et al. (2026) studied this question.
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