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The charge transport in dye-sensitized nanostructured TiO 2 was studied by laser pulse induced photocurrent transients. The experimental curves were compared to simulations using a diffusion model with an initial electron distribution of an exponential decay. The simulations were optimized with respect to the experimental curves giving an apparent diffusion coefficient of 6 × 10 -6 cm 2 /s for the electrons with an electrolyte of 0.1 M KI in propylene carbonate, the potential being +300 mV vs Ag/AgCl in ethanol. The charge transport was highly dependent on electrolyte composition and light intensity.
Solbrand et al. (Fri,) studied this question.