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The molecular structure of the linear C2S and C3S molecules were studied by a quantum chemical method. The calculated rotational constant is 6438 MHz for C2S and 2888 MHz for C3S. After vibrational correction, these values agree closely with experiment. The calculated dipole moments of C2S and C3S are 2.8 D and 3.6 D, respectively. The addition of a carbon atom stabilizes the short carbon-chain monosulfides about 100-160 kcal/mol.
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Akinori Murakami (1990) studied this question.
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