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Carbon dioxide removal from flue gas with a two-stage vacuum pressure swing adsorption (VPSA) process, which uses activated carbon (AC) beads as the adsorbent, was investigated both theoretically and experimentally. First, single-column VPSA experiments were studied for CO 2 /N 2 separation with high CO 2 feed concentration. Then, a two-stage VPSA process composed two columns for each stage was designed, and the effects of different parameters were investigated. The first-stage VPSA unit operates with a four-step Skarstrom cycle, which includes feed pressurization, adsorption, blowdown, and counter-current purge with N 2 . For the second-stage VPSA process, a cycle with feed pressurization, adsorption, pressure equalization, blowdown and pressure equalization was employed. With the proposed two-stage VPSA process, a CO 2 purity of 95.3% was obtained with 74.4% recovery. The total specific power consumption of the two-stage VPSA process is 723.6 kJ/kg-CO 2, while the unit productivity is 0.85 mol-CO 2 /kg·h.
Shen et al. (Sat,) studied this question.