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We investigate the use of a tunable spin-flip Raman laser in infrared absorption spectroscopy. The Raman laser is tunable from 10.9 to 13.0 {μ}m with linearity and resettability of tuning better than {~}4 {}A at {~}12.0 {μ}m. This limit is set by the present measurement capability. A study of the absorption spectrum of NH₃ in the 12.0-{μ}m region shows that the spin-flip Raman laser is superior to a conventional grating spectrometer in attainable resolution.
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Patel et al. (1970) studied this question.
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