Assuming a unique linear periodic lattice for a non-ionic molecular mix-crystal, the lattice frequencies of the translational and rotational modes have been calculated for several concentration ratios of the two components. The observed variation in frequency in such crystals has been explained. The calculations also require that additional frequencies, not yet observed, should appear in Raman and infrared spectra.
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Aggarwal et al. (1951) studied this question.
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