Extensive control over enantiomer populations using achiral light is computationally demonstrated for J, MJ-selected 1,3 dimethylallene. In particular, by altering the detuning of one of three lasers incident on an J, MJ-polarized racemic mixture, one can alter the enantiomeric excess from ≈93% of the L enantiomer to ≈93% of the D enantiomer.
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Gerbasi et al. (2001) studied this question.
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