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August 6, 2026ACS Applied Energy Materials

Enhanced Thermoelectric Performance by Carrier Optimization in Layered SnSe2 with Low Thermal Conductivity

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Authors

ZLZhenqi LiBeihang UniversitySBShulin BaiZhejiang International Studies UniversityDLDongrui LiuBeihang University

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Implication

Randomized trial demonstrates improved thermoelectric performance in layered SnSe2, indicating effective carrier optimization.

Key Points

  • The aim is to enhance the thermoelectric performance of layered SnSe2 by optimizing charge carrier density while maintaining low thermal conductivity.
  • Optimized ambient-temperature electron concentration from 1.0 × 10^19 cm–3 to 5.2 × 10^19 cm–3.
  • Measured peak thermoelectric ZT of ∼1.4 at 723 K in SnSe2 polycrystal.
  • Conducted first-principles computations to analyze thermal transport mechanisms.
  • Achieved significant increase in charge conduction and power factor while keeping total heat conduction at ∼0.6–0.8 W m–1 K–1.
  • Demonstrated that soft interlayer acoustic vibrational modes contribute to suppressed thermal transport.
  • Established carrier optimization within a soft lattice as a strategy for high-efficiency thermoelectric conversion.

Cite This Study

Li et al. (2026) studied this question.

synapsesocial.com/papers/6a74379d764cddc9499d5145https://doi.org/10.1021/acsaem.6c02169
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