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A stepwise four-electron reaction significantly alleviates the thermodynamics reaction barrier for overall water splitting. Regenerated 1D carbon nitride nanowire bundles from tailoring and reassembly of 2D g-C3N4 produce novel physicochemical and optoelectronic properties, which well realize the stepwise four-electron reaction along with a quantum efficiency of 5.2‰ at 420 nm.
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Zhang et al. (2016) studied this question.
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