Infrared dispersion data on liquid CS2 in the wavelength range 2–15 μ have been analyzed according to classical dispersion theory to yield both gas and liquid oscillator strengths for the asymmetric stretching vibration. The calculated gas intensity for this vibration is 7000×1010 cm—1 sec—1 (STP) as compared to directly measured values around 7500×1010. The intensity of the bending vibration of CS2 which has not yet been measured is inferred to be 275×1010 cm—1 sec—1. The CS bond dipole moment is calculated to be 1.24 debye which gives a quadrupole moment in reasonable agreement with experiment.
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Ferguson et al. (1959) studied this question.
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