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The fundamental vibrational frequencies of an isolated chain of trans ‐1,4‐polychloroprene have been calculated. The agreement between the calculated and experimentally observed crystalline frequencies supports the molecular model for the structure of trans ‐1,4‐polychloroprene and the force field employed in the calculations. The results of the normal coordinate analysis indicate that there is essentially no coupling between adjacent translational repeat units of trans ‐1,4‐polychloroprene.
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Tabb et al. (1975) studied this question.
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