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The classical dynamics of intramolecular energy flow caused by potential and Coriolis couplings is studied in various representations. The mapping of the problem onto a perturbed asymmetric rotor is found particularly useful. This representation shows the origin of localization/delocalization of energy as well as factors that determine periodic energy exchange. Good agreement is found between the predictions and numerical calculations.
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Sahm et al. (1989) studied this question.
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