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Uniform multilayer films of polyelectrolytes (charged polymers) that incorporate redox-active polyelectrolytes are demonstrated to be formed by a simple electrostatic layer-by-layer approach. On conducting substrates, the redox sites within these films are addressable by electrochemical methods. This is verified by considering two examples—the electrochromism and electrocatalysis of polyviologen multilayers—to check that the physical properties of these films are modulated by electrochemistry.
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Schlenoff et al. (1998) studied this question.
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