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The synthesis, crystal structure and magnetic properties of the non‐transition metals; Cd(II), Zn(II), Hg(II), Mg(II) and the transition metals; Co(II), Ni(II), Cu(II) complexes with 2‐(4‐pyridyl)‐4,4,5,5‐tetra‐methylimidazolinyl‐l‐oxy‐3‐oxide (NITpPy) are presented. The compounds of free radical NITpPy, HgCl 2 (NITpPy), and Zn(acac) 2 (NITpPy) crystallize in the same monoclinic system of space group C2/c. The magnetic properties of the temperature‐dependent magnetic susceptibility of NITpPy and its metal complexes are discussed according to the Heisenberg model. A weak ferromagnetic coupling in NITpPy and a weak antiferromagnetic coupling in the metal complexes have been revealed.
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Wei et al. (1996) studied this question.
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