Vacuum ultraviolet (VUV) photolysis of N2O immersed in high-pressure Ar has been used to produce O(1S0) at high density. A two-chamber apparatus was used to prevent the effects of electron and ion collision in the experimental volume, thereby providing a much clearer kinetic situation. The gain profile and stimulated emission cross section near 558 nm and the upper-state lifetime were determined for ArO.
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Hughes et al. (1976) studied this question.
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