The theory of nonisothermal, nonstationary diffusion in a two-bulb geometry is corrected and extended. Two major corrections to simple theory are necessary: one for the variation with time of the thermal diffusion ratio, and one for the deviations from a quasistationary state in the connecting tube. All previous treatments of the second correction contain inadequacies serious enough to necessitate revision of many reported diffusion coefficients
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Annis et al. (1969) studied this question.
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