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An attempt is made to obtain frequencies of internal vibrations of some organic molecules by the consideration of certain mechanical systems.The system of three particles is studied assuming the forces of restitution elastic. Certain proportionality constants are determined, using a representative compound, which characterize the single valence bond. Calculated wave-numbers for CO₂, CS₂, CH₂{Cl}₂$, ${C}₂H₅OH are compared with observed data from Raman spectra.
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Robert C. Yates (1930) studied this question.
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