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August 19, 2026Advanced Functional Materials

Tough Hydrophobic Ionogel Fibers via Molecularly Engineered Phase Separation for Multi‐Scenario Sensing

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Authors

LZLunyu ZhaoZWZitong WangYZYanan Zhang

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Overview

Experimental study demonstrates tough hydrophobic ionogel fibers with high stretchability and sensitivity, suggesting broad utility for wearable sensing in extreme environments.

Key Points

  • Develop robust, stretchable, and environmentally tolerant hydrophobic ionogel fibers for flexible strain sensing under harsh conditions.
  • Synthesized hydrophobic ionogel fibers via molecularly engineered polymerization-induced phase separation inspired by biological composites.
  • Embedded rigid hydrogen-bonded polyacrylamide nanophases into an elastic fluoropolymer matrix to construct continuous ion-transport pathways.
  • Assessed mechanical strength, electrical conductivity, self-healing, underwater adhesion, and strain sensing across diverse temperatures, vacuum levels, and humidity conditions.
  • Achieved a fracture strength of 4.5 MPa, toughness of 24.6 MJ/m³, and stretchability of approximately 900%.
  • Demonstrated high strain sensitivity with a gauge factor of 11.5 across extreme operating conditions, including temperatures from -40°C to 100°C, 1.325 kPa vacuum, 98% relative humidity, and underwater immersion.

Cite This Study

Zhao et al. (2026) studied this question.

synapsesocial.com/papers/6a85639d03308d306e2d6dc3https://doi.org/10.1002/adfm.77764
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