Spin-polarized quasiparticle transport in cuprate superconductors

The effects of spin-polarized quasiparticle transport in superconducting YBa₂Cu₃O_7-δ (YBCO) epitaxial films are investigated by means of current injection into perovskite ferromagnet-insulator-superconductor (F-I-S) heterostructures. These effects are compared with the injection of simple quasiparticles into control samples of perovskite nonmagnetic metal-insulator-superconductor (N-I-S). Systematic studies of the critical current density (Jc) as a function of the injection current density (Jᵢₙⱼ), temperature $(T),$ and the thickness (d) of the superconductor reveal drastic differences between the F-I-S and N-I-S heterostructures, with strong suppression of Jc and a rapidly increasing characteristic transport length near the superconducting transition temperature Tc only in the F-I-S samples. The temperature dependence of the efficiency (η≡ΔJc/Jᵢₙⱼ; ΔJc: the suppression of critical current due to finite Jᵢₙⱼ) in the F-I-S samples is also in sharp contrast to that in the N-I-S samples, suggesting significant redistribution of quasiparticles in F-I-S due to the longer lifetime of spin-polarized quasiparticles. Application of conventional theory for nonequilibrium superconductivity to these data further reveal that a substantial chemical potential shift μ* in F-I-S samples must be invoked to account for the experimental observation, whereas no discernible chemical potential shift exists in the N-I-S samples, suggesting strong effects of spin-polarized quasiparticles on cuprate superconductivity. The characteristic times estimated from our studies are suggestive of anisotropic spin relaxation processes, possibly with spin-orbit interaction dominating the c-axis spin transport and exchange interaction prevailing within the CuO₂ planes. Several alternative scenarios attempted to account for the suppression of critical currents in F-I-S samples are also critically examined, and are found to be neither compatible with experimental data nor with the established theory of nonequilibrium superconductivity.