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Complementarity between different techniques (magnetization, HF-HFEPR, FDMRS) and angular-overlap-model calculations allow the precise determination of the spin-Hamiltonian parameters in an isolated octahedral NiII complex (see structure), which exhibits the largest easy axis magnetic anisotropy reported to date (D=−10.1 cm−1, E/|D|=0.02).
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Rogez et al. (2005) studied this question.
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