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The sensitivity of a microwave coherent transient spectrometer has been improved by two orders of magnitude. Rotational transitions in the ground and the vibrational excited states of ν2, ν1, and 2ν2 of OCS are systematically investigated to obtain the transverse relaxation rate constants. The calculation using the Anderson–Tsao–Curnutte theory gives a satisfactory explanation of the observed rotational- and vibrational-state dependence of the rate constants.
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Matsuo et al. (1985) studied this question.
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