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Surface-enhanced Raman scattering from molecular monolayers adsorbed at the aluminum oxide---Ag interface of tunnel junctions has been studied as a function of the junction parameters and surface roughness. The surface-plasmon---polariton contribution to surface-enhanced Raman scattering from this system is quantitatively demonstrated in experiments on samples fabricated on holographic diffraction gratings. The existence of a short-range contribution to the surface-enhanced Raman effect is also shown and compared with the predictions of the modulated surface dipole mechanism of Jha, Kirtley, and Tsang.
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Tsang et al. (1982) studied this question.
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